Cluster dynamics - laser excitation versus ionic collisions

The influence of various excitation mechanisms (lasers, collision with highly charged ions) on the electronic and ionic dynamics of metal clusters is investigated. The tools are TDLDA calculations with simultanous dynamics of the ionic cores. In selected cases, effects beyond TDLDA are included. The results are analyzed in terms of several global observables (number of emitted electrons, energy balance, dipole signal) and of a few detailed ones (distribution of kinetic energies, angular distribution, ionization probabilities). It is found that ionic collision perform very similar to femtosecond lasers with respect to most global observables. The detailed distributions, however, do depende more sensitively on the excitation mechanism and its parameters.




Extreme Fields
3/16/2000